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Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10,   Pages 1354-1371 doi: 10.1007/s11705-022-2286-4

Abstract: With the increasing development of digital devices and electric vehicles, high energy-density rechargeable batteries are strongly required. As one of the most promising anode materials with an ultrahigh specific capacity and extremely low electrode potential, lithium metal is greatly considered an ideal candidate for next-generation battery systems. Nevertheless, limited Coulombic efficiency and potential safety risks severely hinder the practical applications of lithium metal batteries due to the inevitable growth of lithium dendrites and poor interface stability. Tremendous efforts have been explored to address these challenges, mainly focusing on the design of novel electrolytes. Here, we provide an overview of the recent developments of localized high-concentration electrolytes in lithium metal batteries. Firstly, the solvation structures and physicochemical properties of localized high-concentration electrolytes are analyzed. Then, the developments of localized high-concentration electrolytes to suppress the formation of dendritic lithium, broaden the voltage window of electrolytes, enhance safety, and render low-temperature operation for robust lithium metal batteries are discussed. Lastly, the remaining challenges and further possible research directions for localized high-concentration electrolytes are outlined, which can promisingly render the practical applications of lithium metal batteries.

Keywords： high-concentration electrolyte     localized high-concentration electrolyte     lithium metal battery     solidelectrolyte interphase     dendrite    

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Recent advances toward high voltage, EC-free electrolytes for graphite-based Li-ion battery

Tong Zhang, Elie Paillard

Frontiers of Chemical Science and Engineering 2018, Volume 12, Issue 3,   Pages 577-591 doi: 10.1007/s11705-018-1758-z

Abstract: graphite anode operation–also required for high energy density batteries–by stabilizing the electrode/electrolyteThis review covers electrolyte compositions, with the widespread use of additives, the change in mainsalt) concentration, but also reports on graphite protection strategies, by coatings or artificial solidelectrolyte interphase (SEI) or by use of water-soluble binder for electrode processing as these can

Keywords： lithium-ion     electrolyte     solid electrolyte interphase     additives     high voltage     graphite    

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A review on the development of electrolytes for lithium-based batteries for low temperature applications

Frontiers in Energy 2023, Volume 17, Issue 1,   Pages 43-71 doi: 10.1007/s11708-022-0853-5

Abstract: cosolvents, additives, and salts have been researched to fine tune the conductivity, solvation, and solid-electrolyteWith these objectives in mind, tailoring of the electrolyte with higher-capacity materials such as lithiumThis review paper highlights the progression of electrolyte research for low temperature performance

Keywords： electrolyte     lithium-ion     low temperature     aerospace     solid-electrolyte interface    

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The method for the conductivity measurement of electrolyte and electrode materials in solid oxide fuel

He Beibei,Pan Xin,Xia Changrong

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 57-65

Abstract:

The conductive mechanism of crystal material, especially of the solid oxide fuel cell components isSome commonly used measurements for electrolyte and electrode materials, such as total conductivity

Keywords： conduction mechanism     electrolyte     electrode     conductivity     solid oxide fuel cell    

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Ion conduction path in composite solid electrolytes for lithium metal batteries: from polymer rich to

Zhouyu ZHANG, Hao CHEN, Zhenglin HU, Shoubin ZHOU, Lan ZHANG, Jiayan LUO

Frontiers in Energy 2022, Volume 16, Issue 5,   Pages 706-733 doi: 10.1007/s11708-022-0833-9

Abstract: Solid-state electrolytes (SSEs) can address the safety issue of organic electrolyte in rechargeable lithiumComposite solid electrolytes (CSEs) composed of flexible polymers and brittle but more conducting ceramicscan take advantage of the individual system for solid-state lithium metal batteries (SSLMBs).

Keywords： composite solid electrolytes     active filler/framework     ion conduction path     interphase compatibility    

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The composite electrolyte materials for low-temperature solid oxide fuel cell

Xie Fucheng,Wang Cheng,Mao Zongqiang

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 72-76

Abstract:

Solid oxide fuel cell (SOFC) has been extensively identified as one of the most promising energyFunctional composite electrolytes are regarded as the promising electrolyte materials, and the ionThe recent progress in composite electrolyte, the characteristics, type and conductive mechanismof composite electrolyte were introduced in the paper.

Keywords： low-temperature SOFC     composite electrolyte     conductive mechanism    

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Boosting the direct conversion of NHHCO electrolyte to syngas on Ag/Zn zeolitic imidazolate framework

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 9,   Pages 1196-1207 doi: 10.1007/s11705-022-2289-1

Abstract: which were used for the first time for boosting the direct conversion of NH4HCO3 electrolyteIts activity is comparable to that of the CO2-saturated NH4HCO3 electrolyte

Keywords： Ag catalyst     zeolitic imidazolate framework     CO2 electroreduction     ammonium bicarbonate electrolyte    

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Development of metal-supported SOFC

Zhou Yongchuan,Song Shidong,Han Minfang

Strategic Study of CAE 2013, Volume 15, Issue 2,   Pages 27-32

Abstract:

Developing of intermediate temperature (IT) and low temperature (LT) solid oxide fuel cell (SOFC)Recently, MS-SOFC has developed various structures and fabrication process of supporter, electrolyte

Keywords： solid oxide fuel cell     metal-supported SOFC     thin-film electrolyte     thermal cycle     fast start-up    

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Modification of NASICON Electrolyte and Its Application in Real Na-Ion Cells Article

Qiangqiang Zhang, Quan Zhou, Yaxiang Lu, Yuanjun Shao, Yuruo Qi, Xingguo Qi,Guiming Zhong, Yong Yang, Liquan Chen, Yong-Sheng Hu

Engineering 2022, Volume 8, Issue 1,   Pages 170-180 doi: 10.1016/j.eng.2021.04.028

Abstract:

The low ionic conductivity of solid-state electrolytes (SSEs) and the inferior interfacial reliabilitybetween SSEs and solid-state electrodes are two urgent challenges hindering the application of solid-state>MgxSi2PO12 were synthesized using a facile two-step solid-state

Keywords： Solid-state electrolytes     Solid-state sodium batteries     NASICON     Interface     Separator     Coating    

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Effect of electrolyte concentration on the tribological performance of MAO coatings on aluminum alloys

Chao Wang, Jun Chen, Jihua He, Jing Jiang, Qinyong Zhang

Frontiers of Chemical Science and Engineering 2020, Volume 14, Issue 6,   Pages 1065-1071 doi: 10.1007/s11705-019-1909-x

Abstract: In order to investigate the effect of the electrolyte concentration on the properties of MAO coatings

Keywords： aluminum alloy     micro-arc oxidation     coating     electrolyte concentration     tribological performance    

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Interphase precipitation in low carbon Ti-V microalloyed steels

Jia Tao,Wei Jiao,Feng Jie,Zhang Weina,Liu Zhenyu and Wang Guodong

Strategic Study of CAE 2014, Volume 16, Issue 1,   Pages 88-92

Abstract: dilatometer，the sample was held at austenite/ferrite dual- phase temperature region and the Ti-V complex interphaseelectron microscopy （TEM） were employed to analyze the microstructure，especially the morphology of the interphaseThe interphase precipitates exhibit sheet-like distribution，including flat and curved sheets and adopt

Keywords： Ti-V microalloyed steel     interphase precipitation     isothermal phase transformation     TEM    

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Review of characterization and modeling of polymer electrolyte fuel cell catalyst layer: The blessing

Jun HUANG, Zhe LI, Jianbo ZHANG

Frontiers in Energy 2017, Volume 11, Issue 3,   Pages 334-364 doi: 10.1007/s11708-017-0490-6

Abstract: Ionomer impregnation represents a milestone in the evolution of polymer electrolyte fuel cell (PEFC)

Keywords： polymer electrolyte fuel cell     ultra-thin catalyst layer     electrostatic interactions     characterization and    

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Characterization and comparison of organic functional groups effects on electrolyte performance for vanadium

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 9,   Pages 1221-1230 doi: 10.1007/s11705-023-2298-8

Abstract: sulfonic acid, sulfonic acid, amino methane sulfonic acid, and taurine are used to overcome the low electrolyteWhen compared to the pristine electrolyte (0.22 Ah, 5.0 Wh·L–1, 85.0%), the results show thatThe acetic acid electrolyte is more conducive to the low-temperature stability of the V(II) electrolytesub>H group, specifically the coaction of the –NH2 and –SO3H groups, improves electrolyte

Keywords： vanadium redox flow battery     functional groups     organic additives     energy density     stability    

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Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Frontiers in Energy 2017, Volume 11, Issue 3,   Pages 365-373 doi: 10.1007/s11708-017-0500-8

Abstract: Although a thin layer of electrolyte decomposition products is known to form at the cathode surface,The ReaxFFMD simulations reveal that the cathode-electrolyte interface layer is composed of oxidationproducts of electrolyte solvent molecules including aldehydes, esters, alcohols, polycarbonates, andThe oxidation reaction pathways for the electrolyte solvent molecules involve the formation of surfaceAn overall cathode-electrolyte interface reaction scheme is proposed based on the molecular simulation

Keywords： lithium manganese oxide batteries     reactive force field (ReaxFF)     cathode-electrolyte interface layer     molecular    

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Recent Advances in Energy Chemical Engineering of Next-Generation Lithium Batteries Review

Xue-Qiang Zhang, Chen-Zi Zhao, Jia-Qi Huang, Qiang Zhang

Engineering 2018, Volume 4, Issue 6,   Pages 831-847 doi: 10.1016/j.eng.2018.10.008

Abstract:

Rechargeable lithium-ion batteries (LIBs) afford a profound impact on our modern daily life. However, LIBs are approaching the theoretical energy density, due to the inherent limitations of intercalation chemistry; thus, they cannot further satisfy the increasing demands of portable electronics, electric vehicles, and grids. Therefore, battery chemistries beyond LIBs are being widely investigated. Next-generation lithium (Li) batteries, which employ Li metal as the anode and intercalation or conversion materials as the cathode, receive the most intensive interest due to their high energy density and excellent potential for commercialization. Moreover, significant progress has been achieved in Li batteries attributed to the increasing fundamental understanding of the materials and reactions, as well as to technological improvement. This review starts by summarizing the electrolytes for next-generation Li batteries. Key challenges and recent progress in lithium-ion, lithium–sulfur, and lithium–oxygen batteries are then reviewed from the perspective of energy and chemical engineering science. Finally, possible directions for further development in Li batteries are presented. Next-generation Li batteries are expected to promote the sustainable development of human civilization.

Keywords： Lithium-ion batteries     Lithium–sulfur batteries     Lithium–oxygen batteries     Lithium metal     Solid-state batteries     Battery chemistry     Electrolyte    

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Title Author Date Type Operation

Localized high-concentration electrolytes for lithium metal batteries: progress and prospect

Journal Article

Recent advances toward high voltage, EC-free electrolytes for graphite-based Li-ion battery

Tong Zhang, Elie Paillard

Journal Article

A review on the development of electrolytes for lithium-based batteries for low temperature applications

Journal Article

The method for the conductivity measurement of electrolyte and electrode materials in solid oxide fuel

He Beibei,Pan Xin,Xia Changrong

Journal Article

Ion conduction path in composite solid electrolytes for lithium metal batteries: from polymer rich to

Zhouyu ZHANG, Hao CHEN, Zhenglin HU, Shoubin ZHOU, Lan ZHANG, Jiayan LUO

Journal Article

The composite electrolyte materials for low-temperature solid oxide fuel cell

Xie Fucheng,Wang Cheng,Mao Zongqiang

Journal Article

Boosting the direct conversion of NHHCO electrolyte to syngas on Ag/Zn zeolitic imidazolate framework

Journal Article

Development of metal-supported SOFC

Zhou Yongchuan,Song Shidong,Han Minfang

Journal Article

Modification of NASICON Electrolyte and Its Application in Real Na-Ion Cells

Qiangqiang Zhang, Quan Zhou, Yaxiang Lu, Yuanjun Shao, Yuruo Qi, Xingguo Qi,Guiming Zhong, Yong Yang, Liquan Chen, Yong-Sheng Hu

Journal Article

Effect of electrolyte concentration on the tribological performance of MAO coatings on aluminum alloys

Chao Wang, Jun Chen, Jihua He, Jing Jiang, Qinyong Zhang

Journal Article

Interphase precipitation in low carbon Ti-V microalloyed steels

Jia Tao,Wei Jiao,Feng Jie,Zhang Weina,Liu Zhenyu and Wang Guodong

Journal Article

Review of characterization and modeling of polymer electrolyte fuel cell catalyst layer: The blessing

Jun HUANG, Zhe LI, Jianbo ZHANG

Journal Article

Characterization and comparison of organic functional groups effects on electrolyte performance for vanadium

Journal Article

Chemical composition and formation mechanisms in the cathode-electrolyte interface layer of lithium manganese

Sahithya REDDIVARI, Christian LASTOSKIE, Ruofei WU, Junliang ZHANG

Journal Article

Recent Advances in Energy Chemical Engineering of Next-Generation Lithium Batteries

Xue-Qiang Zhang, Chen-Zi Zhao, Jia-Qi Huang, Qiang Zhang

Journal Article